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Abstract Massive stars are a major source of chemical elements in the cosmos, ejecting freshly produced nuclei through winds and core-collapse supernova explosions into the interstellar medium. Among the material ejected, long-lived radioisotopes, such as⁶⁰Fe (iron) and²⁶Al (aluminum), offer unique signs of active nucleosynthesis in our galaxy. There is a long-standing discrepancy between the observed⁶⁰Fe/²⁶Al ratio by γ-ray telescopes and predictions from supernova models. This discrepancy has been attributed to uncertainties in the nuclear reaction networks producing⁶⁰Fe, and one reaction in particular, the neutron-capture on⁵⁹Fe. Here we present experimental results that provide a strong constraint on this reaction. We use these results to show that the production of⁶⁰Fe in massive stars is higher than previously thought, further increasing the discrepancy between observed and predicted⁶⁰Fe/²⁶Al ratios. The persisting discrepancy can therefore not be attributed to nuclear uncertainties, and points to issues in massive-star models. 

The synthesis of heavy elements in supernovae is affected by low-energy $(n,p)$and $(p,n)$reactions on unstable nuclei, yet experimental data on such reaction rates are scarce. The SECAR (SEparator for CApture Reactions) recoil separator at FRIB (Facility for Rare Isotope Beams) was originally designed to measure astrophysical reactions that change the mass of a nucleus significantly. We used a novel approach that integrates machine learning with ion-optical simulations to find an ion-optical solution for the separator that enables the measurement of $(p,n)$reactions, despite the reaction leaving the mass of the nucleus nearly unchanged. A new measurement of the ${}^{58}\mathrm{Fe}(p,n){}^{58}\mathrm{Co}$reaction in inverse kinematics with a $3.66\pm 0.12$MeV/nucleon ${}^{58}\mathrm{Fe}$beam (corresponding to $3.69\pm 0.12$MeV proton energy in normal kinematics) yielded a cross-section of $20.3\pm 6.3$ mb and served as a proof of principle experiment for the new technique demonstrating its effectiveness in achieving the required performance criteria. This novel approach paves the way for studying astrophysically important $(p,n)$reactions on unstable nuclei produced at FRIB. Published by the American Physical Society2025